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Decision Tree and K-Means Analysis of Raman Spectra for Edible Oils: A Physics-Informed AI Approach

arXiv:2608.20440v1 Announce Type: new Abstract: Authentication of edible oils in processed foods is important for food quality, fraud prevention, and regulatory compliance. This study establishes an integrated Raman spectroscopy and machine-learning framework that links intrinsic spectral organization, interpretable classification, and Physics-Informed Artificial Intelligence (PI-AI). Five edible oils were investigated in pure form and within a fried-potato-chip matrix using t-SNE, K-means clustering, Decision Trees, and Non-Negative Least Squares (NNLS)-based spectral decomposition. Unsupervised analyses revealed substantially stronger class organization and separability in pure oils, whereas food-matrix effects introduced pronounced spectral overlap. Decision Trees achieved 100% classification accuracy for pure oils using only four Raman variables from the original 1866-feature spectral space. These four variables, consistently identified by both pre-pruned and post-pruned models, represented only approximately 0.21% of the available spectral information while retaining perfect test-set performance. For matrix-containing samples, NNLS-based PI-AI spectral decomposition substantially improved classification by separating oil-related signatures from paper and potato contributions. Optimized post-pruned models achieved accuracies of 86.4% and 85.4% for paper-subtracted and paper-plus-potato-subtracted datasets, respectively, while reducing the number of important Raman variables to only five and four. The compact four-feature representation further reduced the data footprint by 99.44% without loss of classification accuracy. Collectively, these findings demonstrate that accurate Raman-based oil identification can be achieved through physically meaningful, highly compact, and interpretable spectral representations, providing a promising foundation for Frugal AI, Edge AI, portable sensing, and embedded food-quality monitoring.

SourcearXiv Machine LearningAuthor: Amrita Shaw, Chandrasekar S. N., Sai Muthukumar V., Jhinuk Gupta, Deepak L. N. Kallepalli

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[Submitted on 20 Aug 2026]

Title:Decision Tree and K-Means Analysis of Raman Spectra for Edible Oils: A Physics-Informed AI Approach

View a PDF of the paper titled Decision Tree and K-Means Analysis of Raman Spectra for Edible Oils: A Physics-Informed AI Approach, by Amrita Shaw and 4 other authors

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Abstract:Authentication of edible oils in processed foods is important for food quality, fraud prevention, and regulatory compliance. This study establishes an integrated Raman spectroscopy and machine-learning framework that links intrinsic spectral organization, interpretable classification, and Physics-Informed Artificial Intelligence (PI-AI). Five edible oils were investigated in pure form and within a fried-potato-chip matrix using t-SNE, K-means clustering, Decision Trees, and Non-Negative Least Squares (NNLS)-based spectral decomposition. Unsupervised analyses revealed substantially stronger class organization and separability in pure oils, whereas food-matrix effects introduced pronounced spectral overlap. Decision Trees achieved 100% classification accuracy for pure oils using only four Raman variables from the original 1866-feature spectral space. These four variables, consistently identified by both pre-pruned and post-pruned models, represented only approximately 0.21% of the available spectral information while retaining perfect test-set performance. For matrix-containing samples, NNLS-based PI-AI spectral decomposition substantially improved classification by separating oil-related signatures from paper and potato contributions. Optimized post-pruned models achieved accuracies of 86.4% and 85.4% for paper-subtracted and paper-plus-potato-subtracted datasets, respectively, while reducing the number of important Raman variables to only five and four. The compact four-feature representation further reduced the data footprint by 99.44% without loss of classification accuracy. Collectively, these findings demonstrate that accurate Raman-based oil identification can be achieved through physically meaningful, highly compact, and interpretable spectral representations, providing a promising foundation for Frugal AI, Edge AI, portable sensing, and embedded food-quality monitoring.

Comments: 36 pages, 11 figures, 2 tables, 9 supplementary figures

Subjects:

Machine Learning (cs.LG); Artificial Intelligence (cs.AI)

Cite as: arXiv:2608.20440 [cs.LG]

(or arXiv:2608.20440v1 [cs.LG] for this version)

https://doi.org/10.48550/arXiv.2608.20440

arXiv-issued DOI via DataCite (pending registration)

Submission history

From: Deepak Kallepalli Dr. [view email] [v1] Thu, 20 Aug 2026 14:07:32 UTC (1,814 KB)

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